Abstract
In this study, the effects of increasing sonication times (0 min, 60 min, 120 and 150 min), sonication temperatures (25oC, 30oC and 60oC), increasing titanium dioxide (TiO2) (0.1 mg/L, 0.5 mg/L, 10 and 20 mg/L), sodium chloride (NaCl) (1 g/L, 2.5 and 15 g/L), ferrous ion (Fe+2) (2 mg/L, 8 and 20 mg/L) and ferric ion (Fe+3) (10 mg/L, 20 and 50 mg/L) concentrations on the dissolved chemical oxygen demand (CODdis), total organic carbon (TOC) and total polycyclic aromatic hydrocarbons (PAH) removal efficiencies were monitored at a sonication frequency of 35 kHz and a sonication power of 640 W for a raw petrochemical industry wastewater (PCI ww). As the sonication time and temperature were increased from 60 to 120 and 150 min, and from 25 oC to 30 oC and to 60 oC, the CODdis, total PAH and TOC yields increased from around 52-58% and 69%-72% to 80-87% and 78%-90%. The maximum CODdis, total PAH and TOC yields were obtained with 20 mg/l TiO2, 15 mg/l NaCl, 20 mg/L Fe+2 and with 50 mg/L Fe+3, particularly after 150 min sonication at 60 oC. However, it is important to note that after 150 min sonication in the samples free of the chemicals mentioned above, in other words, in the samples with only sonication exhibited high yields as is the samples added the chemicals. After sonication with the chemicals, the EC50 values decreased significantly versus sonication times. The maximum Daphnia magna acute toxicity removal yield was 99.91% at NaCl=1 g/L at 60oC after 150 min sonication.References
Suslick KS, Hammerton DA, Cline Jr. RE. The sonochemical hot spot. J Am Chem Soc 1986; 108(25): 5641-50. https://doi.org/10.1021/ja00278a055
Suslick KS. Sonoluminescence and sonochemistry. Phil Trans Roy Soc London A 2000; 361(2): 342-68.
Wheat PE, Tumeo MA. Ultrasound induced aqueous polycyclic aromatic hydrocarbon reactivity. Ultrason Sonochem 1997; 4(1): 55-9. https://doi.org/10.1016/S1350-4177(96)00017-X
Cataldo F. Ultrasound-induced cracking and pyrolysis of some aromatic and naphthetic hydrocarbons. Ultrason Sonochem 2000; 7(1): 35-43. https://doi.org/10.1016/S1350-4177(99)00019-X
Grishchenkov GV, Townsend RT, McDonald TJ, Autenrieth RL, Bonner JS, Boronin AM. Degradation of petroleum hydrocarbons by facultative anaerobic bacteria under aerobic and anaerobic conditions. Process Biochem 2000; 35(9): 889-96. https://doi.org/10.1016/S0032-9592(99)00145-4
Huang W, Tang X, Felner I, Koltypin Y, Gedanken A. Preparation and characterization of FexOy - TiO2 via sonochemical synthesis. Mater Res Bull 2002; 37(10): 1721-35. https://doi.org/10.1016/S0025-5408(02)00821-8
Banjoo DR, Nelson PR. Improved ultrasonic extraction procedure for the determination of polycyclic aromatic hydrocarbons in sediments. J Chromatogr A 2005; 1066(1-2): 9-18. https://doi.org/10.1016/j.chroma.2005.01.033
David B. Sonochemical degradation of PAH in aqueous solution. Part I: Monocomponent PAH solution. Ultrason Sonochem 2009; 16(2): 260-65. https://doi.org/10.1016/j.ultsonch.2008.07.013
Benabdallah El-Hadj T, Dosta T, Marquez-Serrano J, Mata- Alvaez R. Effect of ultrasound pretreatment in mesophilic and thermophilic anaerobic digestion with emphasis on naphthalene and pyrene removal. Water Res 2007; 41(1): 87-94. https://doi.org/10.1016/j.watres.2006.08.002
Taylor JE, Cook BB, Tarr MA. Dissolved organic matter inhibition of sonochemical degradation of aqueous polycyclic aromatic hydrocarbons. Ultrason Sonochem 1999; 6(4): 175-83. https://doi.org/10.1016/S1350-4177(99)00015-2
Hua L, Wu W-X, Liu Y-X, Tientchen CM, Chen Y-X. Heavy metals and PAHs in sewage sludge from twelve wastewater treatment plants in Zhejiang Province. Biomed Environ Sci 2008; 21(4): 345-52. https://doi.org/10.1016/S0895-3988(08)60053-7
Laughrey Z, Bear E, Jones R, Tarr MA. Aqueous sonolytic decomposition of polycyclic aromatic hydrocarbons in the presence additional dissolved species. Ultrason Sonochem 2007; 8(4): 353-57. https://doi.org/10.1016/S1350-4177(00)00080-8
Busetti F, Heitz A, Cuomo M, Badoer S, Traverso P. Determination of sixteen polycyclic aromatic hydrocarbons in aqueous and solid samples from an Italian wastewater treatment plant. J Chromatogr A 2006; 1102(1-2): 104-15. https://doi.org/10.1016/j.chroma.2005.10.013
Pathak H, Kantharia D, Malpani A, Madamwar D. Naphthalene degradation by Pseudomonas sp. HOB1: In vitro studies and assessment of naphthalene degradation efficiency in simulated microcosms. Water Res 2008; 45(1): 45-53.
Sanchez-Brunete C, Miguel E, Tadeo JL. Analysis of 27 polycyclic aromatic hydrocarbons by matrix solid-phase dispersion and isotope dilution gas chromatography-mass spectrometry in sewage sludge from the Spain area of Madrid. J Chromatogr A 2007; 1148(2): 219-27. https://doi.org/10.1016/j.chroma.2007.03.026
Badin A-L, Faure P, Bedel J-P, Delolme C. Distribution of organic pollutants and natural organic matter in urban storm water sediments as a function of grain size. Sci Total Environ 2008; 403(1-3): 178-87. https://doi.org/10.1016/j.scitotenv.2008.05.022
Zhang G, He J, Zhang P, Zhang J. Ultrasonic reduction of excess sludge from activated sludge system II: Urban sewage sludge treatment. J Hazard Mater 2009; 164(2-3): 1105-09. https://doi.org/10.1016/j.jhazmat.2008.09.015
Luque de Castro MD, Priego-Capote F. Ultrasound-assisted preparation of liquid samples. Talanta 2007; 72(2): 321-34. https://doi.org/10.1016/j.talanta.2006.11.013
Kim IK, Huang CP, Chiu PC. Sonochemical decomposition of dibenzothiophene in aqueous solution. Water Res 2001; 35(18): 4370-78. https://doi.org/10.1016/S0043-1354(01)00176-2
Psillakis E, Goula G, Kalogerakis N, Mantzavinos D. Degradation of polcyclic aromatic hydrocarbons in aqueous solutions by ultrasonic irradiation. J Hazard Mater B 2004; 108(1-2): 95-102. https://doi.org/10.1016/j.jhazmat.2004.01.004
APHA, AWWA, WEF, Standard methods for the examination of water and wastewater. (18th ed.). Washington, DC, USA, 2005.
National Library of Medicine (NLM), Specialized Information Services (SIS), Toxnet, Hazardous Substance Data Bank (HSDB). Retrieved April 10, (2008), from http://toxnet.nlm.nih.gov
Wang J, Ma T, Zhang Z, Zhang X, Jiang Y, Dong D. Investigation on the sonocatalytic degradation of parathion in the presence of nanometer rutile titanium dioxide (TiO2) catalysis. J Hazard Mater B 2006; 137(2): 972-80. https://doi.org/10.1016/j.jhazmat.2006.03.022
Yim B, Yoo Y, Maeda Y. Sonolysis of alkylphenols in aqueous solution with Fe(II) and Fe(III). Chemosphere 2003; 50(8): 1015-23. https://doi.org/10.1016/S0045-6535(02)00665-3
Liu G, Li X, Zhao J, Hidaka H, Serpone N. Photooxidation pathway of sulforhodamine-B.Dependence on the adsorption mode on TiO2 exposed to visible light radiation. Environ Sci Technol 2000; 34(18): 3982-90. https://doi.org/10.1021/es001064c
Sunartio D, Ashokkumar M, Grieser F. Study of the coalescence of acoustic bubbles as a function of frequency, power, and water-soluble additives. J Am Chem Soc 2007; 129(18): 6031-36. https://doi.org/10.1021/ja068980w
Wu Z, Ondruschka B. Roles hydrophobicity and volatility of organic substrates on sonolytic kinetics in aqueous solutions. J Phys Chem 2005; 109(29): 6521-26. https://doi.org/10.1021/jp051768e
Bremmer DH, Di Carlo S, Chakinala AG, Cravotto G. Mineralisation of 2,4-dichlorophenoxyacetic acid by acoustic or hydrodynamic cavitation in conjunction with the advanced Fenton process. Ultrason Sonochem 2008; 15(4): 416-419. https://doi.org/10.1016/j.ultsonch.2007.06.003
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